The Development of Neutron-Physical Model for Two-Zone Research Subcritical Reactor for Nuclear Waste Transmutation

V. I. Gulik1, V. M. Pavlovych2

1Institute for Safety Problems of Nuclear Power Plants, NAS of Ukraine, 12, Lysogirska st., Kyiv, 03028, Ukraine
2Institute for Nuclear Research of NAS, 47, Nauky av., Kyiv, 03680, Ukraine

DOI: doi.org/10.31717/2311-8253.19.1.1

Abstract

The creation of small-scale research subcritical reactors is necessary, in particular, for the development of the technology for nuclear waste transmutation in Accelerator Driven Systems. The construction of such facilities will allow the development of the technology of nuclear waste transmutation without constructing an expensive industrial scale subcritical reactor. The low-cost neutron generator can serve as a driver for such research subcritical reactors. A two-zone model of subcritical system driven by high-intensity neutron generator is proposed in this work. The proposed system can use two separated cores with different neutron spectra: fast and thermal. This paper also represents the main stages of the proposed model of two-zone subcritical reactor development. The results of simulations, aimed at optimizing of the geometry and fuel composition of the two-zone subcritical system, performed in Serpent and MCNP codes are presented. An overview of the analysis of different facilities that can be used as an external neutron source for subcritical reactor is shown, however a high-intensity neutron generator based on D-T reaction was chosen as the optimal neutron source for low-cost research subcritical reactor for investigation of nuclear waste transmutation. Generally, it is observed that the two-zone subcritical system can effectively amplify neutron flux from external neutron sources.

Keywords: Accelerator Driven Systems, subcritical system, transmutation of nuclear waste, optimization of subcritical core.

References

1. IAEA-TECDOC-985. Accelerator Driven Systems: Energy Generation and Transmutation of Nuclear Waste. Status report. Vienna: IAEA, 1997, 482 p.

2. A European Roadmap for Developing Accelerator Driven Systems (ADS) for Nuclear Waste Incineration. The European Technical Working Group on ADS, 2001,145 p.

3. Salvatores M. (2006) Fuel Cycle Strategies for the Sustainable Development of Nuclear Energy: The Role of Accelerator Driven Systems. Nuclear Instruments and Methods in Physics Research A, vol. 562, pp. 578-584.

4. Taczanowski S. (2003) Transmutations of Nuclear Waste in Accelerator-Driven Subcritical Systems. Applied Energy, vol. 75, pp. 97-117.

5. Salvatores M. (2002) The Physics of Transmutation in Critical or Subcritical Reactors. C. R. Physique, vol. 3, pp. 999-1012.

6. Salvatores M. (2002) Transmutation: Issues, Innovative Options and Perspectives. Progress in Nuclear Energy, vol. 40, pp. 375-402.

7. Yang W. S„ Kim Y„ Hill R. N„ Taiwo T. A., Khalil H. S. (2004) Long-Lived Fission Product Transmutation Studies. Nuclear Science and Engineering, vol. 146, pp. 291-318.

8. Jongen Y. et al. (2002) High-Intensity Cyclotrons for Radioisotope Production and Accelerator Driven Systems. Nuclear Physics, vol. 701, pp. 100-103. doi: 10.1016/S0375-9474(01)01555-X.

9. Abderrahim H., Baeten R, Bruyn D., Fernandez R. (2012) MYRRHA – A Multi-Purpose Fast Spectrum Research Reactor. Energy Conversion and Management, vol. 63, pp. 4-10. https://doi.Org/10.1016/j.enconman.2012.02.025.

10. Gohar Y. et al. (2006) Accelerator-Driven Subcritical Facility: Conceptual Design Development. Nuclear Instruments and Methods in Physics Research A, vol. 562, pp. 870-874.

11. Zhong Z., Gohar Y, Talamo A. (2011) Analysis of Fuel Management in the KIPT Neutron Source Facility. Annals of Nuclear Energy, vol. 5, pp. 1014-1022.
12. Verbeke J. M., Leung K. N., Vujic J. (2000) Development of a Sealed-Accelerator-Tube Neutron Generator. Applied Radiation and Isotopes, vol. 53, pp. 801-809.

13. Markovskij D. V. et al. (2001) Experimental Activation Study of Some Russian Vanadium Alloys with 14-MeV Neutrons at SNEG-13 Facility. Fusion Engineering and Design, vol. 58-59, pp. 591-594.

14. Sadowski M. J., Scholz M. (2003) Comments on Status of Plasma Focus Research. Proc. Int. Workshop “Dense Magnetized Plasmas” (Warsaw, Poland, November 25-26, 2003).

15. Talamo A., Gohar Y, Sadovich S., Kiyavitskaya H., Bournos V, Fokov Y, Routkovskaya C. (2014) High enriched to low enriched fuel conversion in YALINA Booster facility. Progress in Nuclear Energy, vol. 70, pp. 43-53.

16. Stacey W. M. (2001) Capabilities of a DT Tokamak Fusion Neutron Source for Driving a Spent Nuclear Fuel Transmutation Reactor. Nuclear Fusion, vol. 41, pp. 135-154.

17. Daniel H., Petrov Yu. V. (1996) Subcritical Fission Reactor Driven by the Low Power Accelerator. Nuclear Instruments and Methods in Physics Research A, vol. 373, pp. 31-134.

18. Kolomiec N. F. (1985) Investigation and Development of Metal-Tritium Neutron-Produced Targets for Accelerators of charged particles (Ph.D. thesis). Kyiv, Institute for Nuclear Research, 156 p.

19. Gulik V. I. (2012) The Model of Two-zone Research Subcritical Nuclear Reactor driven by High-Intensity Neutron Generator (Ph.D. thesis). Kyiv, Institute for Nuclear Research, 143 p.

20. Babenko V. A., Gulik V. F, Jenkovszky L. L., et al. (2005) Study of One-zone Subcritical Amplifier of Neutron Flux Involving Enriched Uranium. Problems of Atomic Science and Technology, vol. 45, no. 6, pp. 122-126.

21. Babenko V. A., Gulik V. I., Jenkovszky L. L., Pavlovych V. M., Pupirina E. A. (2006) On the Subcritical Amplifier of Neutron Flux Based on Enriched Uranium. In: Cechâk T., Jenkovszky L., Karpenko I. (eds.) Nuclear Science and Safety in Europe. Springer Heidelberg, pp. 253-263. doi: 10.1007/978-1-4020-4965-1_21.

22. Gulik V. I., Pavlovich V. N., Pupirina E. A., Babenko V. A. (2006) The Research Subcritical Reactor. Proc. Int. Conf. “Research Reactors in 21st century” (Moscow, Russia, June 20-23, 2006).

23. Briesmeister J. MCNP-A General Monte Carlo Code N-Particle Transport Code Version 4A, LA-12625. Los Alamos National Laboratory, 1993.

24. Babenko V. O., Gulik V. I., Pavlovych V. M., Pupirina O. M. (2006) Two-zone subcritical nuclear reactors. Problems of Nuclear Power Plants’ Safety and of Chornobyl, vol. 6, pp. 8-15.

25. Babenko V O., Gulik V I., Pavlovych V M. (2008) The Research Subcritical Reactor. Nuclear Physics and Atomic Energy, vol. 9, no. 1, pp. 56-61.

26. Babenko V. O., Gulik V. I., Pavlovych V. M. (2010) The New Research Subcritical Reactor driven by a High-intensity Neutron Generator for Transmutation of the Nuclear Waste. Proc. Int. Conf. “WM2010” (Phoenix, Arizona, US, 7-11 March, 2010).

27. Babenko V. O., Gulik V. I., Pavlovych V. M. (2012) Modeling of Two-zone Accelerator-Driven Systems. Nuclear Physics and Atomic Energy, vol. 13, no. 3, pp. 266-275.

28. Babenko V. O., Gulik V. I., Pavlovych V. M., Rybalova A. P. (2011) About Possibility of Nuclear Waste Transmutation in Subcritical System Driven by High-Intensity Neutron Generator. Problems of Nuclear Power Plants’ Safety and of Chornobyl, vol. 16, pp. 8-16.

29. Babenko V. O., Gulik V. I., Pavlovych V. M. (2012) The Transmutation of Nuclear Waste in the Two-Zone Subcritical System Driven by High-Intensity Neutron Generator. Proc. Int. Conf. “WM2012” (Phoenix, Arizona, US, February 26 -March 1, 2012).

30. Leppânen J., Pusa M., Viitanen T., Valtavirta V., Kaltiaisenaho T. (2015) The Serpent Monte Carlo code: Status, development and applications in 2013. Annals of Nuclear Energy, vol. 82, pp. 142-150.

31. Gulik V., Tkaczyk A. H. (2013) Optimization of Geometry, Material and Economic Parameters of a Two-Zone Subcritical Reactor for Transmutation of Nuclear Waste with SERPENT Monte Carlo Code. Proc. Int. Conf. Supercomputing in Nuclear Applications & Monte Carlo (SNA&MC2013) (Paris, France, October 27-31, 2013).

32. Gulik V., Tkaczyk A. H. (2014) Cost Optimization of ADS Design: Comparative Study of Externally Driven Heterogeneous and Homogeneous Two-Zone Subcritical Reactor Systems. Nuclear Engineering and Design, vol. 270, pp. 133-142.

Full Text (PDF)


Published
2019-05-31


If the article is accepted for publication in the journal «Industrial Heat Engineering» the author must sign an agreement on transfer of copyright. The agreement is sent to the postal (original) or e-mail address (scanned copy) of the journal editions.

Authors retain copyright and grant the journal right of first publication with the work simultaneously licensed under a  Creative Commons Attribution License International CC-BY that allows others to share the work with an acknowledgement of the work’s authorship and initial publication in this journal.

Insert math as
Block
Inline
Additional settings
Formula color
Text color
#333333
Type math using LaTeX
Preview
\({}\)
Nothing to preview
Insert